Frequency-noise measurements of optical frequency combs by multiple fringe-side discriminator

open5noThe frequency noise of an optical frequency comb is routinely measured through the hetherodyne beat of one comb tooth against a stable continuous-wave laser. After frequency-to-voltage conversion, the beatnote is sent to a spectrum analyzer to retrive the power spectral density of the frequency noise. Because narrow-linewidth continuous-wave lasers are available only at certain wavelengths, heterodyning the comb tooth can be challenging. We present a new technique for direct characterization of the frequency noise of an optical frequency comb, requiring no supplementary reference lasers and easily applicable in all spectral regions from the terahertz to the ultraviolet. The technique is based on the combination of a low finesse Fabry-Perot resonator and the so-called "fringe-side locking" method, usually adopted to characterize the spectral purity of single-frequency lasers, here generalized to optical frequency combs. The effectiveness of this technique is demonstrated with an Er-fiber comb source across the wavelength range from 1 to 2 μm.Coluccelli, Nicola; Cassinerio, Marco; Gambetta, Alessio; Laporta, Paolo; Galzerano, GianlucaColuccelli, Nicola; Cassinerio, Marco; Gambetta, Alessio; Laporta, Paolo; Galzerano, Gianluc

The optical frequency comb fibre spectrometer

Optical frequency comb sources provide thousands of precise and accurate optical lines in a single device enabling the broadband and high-speed detection required in many applications. A main challenge is to parallelize the detection over the widest possible band while bringing the resolution to the single comb-line level. Here we propose a solution based on the combination of a frequency comb source and a fibre spectrometer, exploiting all-fibre technology. Our system allows for simultaneous measurement of 500 isolated comb lines over a span of 0.12 THz in a single acquisition; arbitrarily larger span are demonstrated (3,500 comb lines over 0.85 THz) by doing sequential acquisitions. The potential for precision measurements is proved by spectroscopy of acetylene at 1.53 μm. Being based on all-fibre technology, our system is inherently low-cost, lightweight and may lead to the development of a new class of broadband high-resolution spectrometers

47-fs Kerr-lens mode-locked Cr:ZnSe laser with high spectral purity

We report on a room-temperature Kerr-lens mode-locked Cr:ZnSe femtosecond laser operating at around 2.4 µm emission wavelength. Self-starting nearly transform-limited pulse trains with a minimum duration of 47 fs, corresponding to six optical cycles, and average output power of 0.25 W are obtained with repetition frequencies in the range from 140 to 300 MHz. The femtosecond pulse train is characterized by high-spectral purity and low time jitter

Diode-pumped passively mode-locked Yb:YLF laser.

We demonstrate passive mode-locking by means of a semiconductor saturable-absorber mirror in a diode-pumped Yb:YLF laser. We present crystal growth process, spectroscopic measurements, and investigation of mode-locking performance. Pulse trains with minimum duration of 196 fs, average power of 54 mW and a repetition rate of 55 MHz were obtained. The optical spectrum, centered at 1028 nm, has a 7.1-nm bandwidth leading to nearly transform-limited pulses. (C) 2008 Optical Society of America

Broadband Fourier-transform coherent Raman spectroscopy with an ytterbium fiber laser.

We demonstrate a Fourier transform (FT) coherent anti-Stokes Raman scattering (CARS) spectroscopy system based on fiber technology with ultra-broad spectral coverage and high-sensitivity. A femtosecond ytterbium fiber oscillator is amplified and spectrally broadened in a photonic crystal fiber to synthesize pulses with energy of 14 nJ at 1040 nm, that are compressed to durations below 20 fs. The resulting pulse train is coupled to a FT-CARS interferometer enabling measurement of high-quality CARS spectra with Raman shifts of ~3000 cm−1 and signal to noise ratio up to 240 and 690 with acetonitrile and polystyrene samples, respectively, for observation times of 160 µs; a detection limit of one part per thousand is demonstrated with a cyanide/water solution. The system has the potential to detect trace contaminants in water as well as other broadband high-sensitivity CARS spectroscopy applications

Fiber-format dual-comb coherent Raman spectrometer

We demonstrate a fiber-format system for dual-comb coherent anti-Stokes Raman scattering spectroscopy. The system is based on two ytterbium fiber (Yb) femtosecond lasers at repetition frequencies of 94 MHz, a Yb amplifier, and a photonic crystal fiber for spectral broadening and generation of pulses with a central wavelength of 1040 nm and durations in the sub-20-fs regime. We observed Raman spectra of acetonitrile and ethyl acetate with spectral coverage from 100 to 1300  cm-1, resolution of 8  cm-1, and a signal-to-noise ratio of around 100, when averaging over 10 acquisitions. The design is suitable for implementing portable dual-comb coherent Raman spectrometers

250-MHz synchronously pumped optical parametric oscillator at 2.25-2.6 {\mu}m and 4.1-4.9 {\mu}m

A compact and versatile femtosecond mid-IR source is presented, based on an optical parametric oscillator (OPO) synchronously pumped by a commercial 250-MHz Er:fiber laser. The mid-IR spectrum can be tuned in the range 2.25-2.6 \mu m (signal) and 4.1-4.9 \mu m (idler), with average power from 20 to 60 mW. At 2.5 \mu m a minimum pulse duration of 110 fs and a power of 40 mW have been obtained. Active stabilization of the OPO cavity length has been achieved in the whole tuning range

Standoff detection of bacterial spores by field deployable coherent Raman spectroscopy

: Vibrational spectroscopies offer great potential for standoff detection of chemical and biological warfare agents, avoiding contamination to the operator and equipment. Among them, particularly promising is Coherent anti-Stokes Raman scattering (CARS) spectroscopy, using synchronized pump/Stokes laser pulses to set up a vibrational coherence of target molecules at a laser focus, which is read by further interaction with a probe pulse, resulting in the emission of a coherent beam detectable at a distance. CARS has previously demonstrated the capability to detect bacterial spores based on the Raman spectrum of the characteristic molecule calcium dipicolinate (CaDPA); however, a complex and bulky laser technology, which is only suitable for a laboratory environment, was employed. Here we develop a broadband CARS setup based on a compact, industrial grade ytterbium laser system. We demonstrate high signal-to-noise ratio detection of Bacillus atrophaeus spores at a concentration of 105 cfu/mm2, at a standoff distance of 1 m, and an acquisition time of 1 s. Our system, which combines chemical specificity and sensitivity along with improved ruggedness and portability, paves the way to a new generation of instruments for real-world standoff detection of chemical and biological threats

Mid-IR tunable CW and passively Q-switched laser operation of Dy-doped fluoride fiber

We report a comprehensive characterization of tunable continuous-wave (CW) and passive Q-switching laser performance of Dy-doped zirconium fluoride fiber emitting around 3 mu m. The in-band pumped CW laser operation is investigated for pump wavelengths varying from 2.7 mu m to 2.825 mu m, for fiber lengths ranging from 0.4 m to 2 m, and for output coupling efficiency from 10% to 50%, leading to a maximum laser slope efficiency of 44% and a tuning range larger than 300 nm. With Findlay-Clay analysis and Rigrod analyses, optimal cavity parameters are retrieved, paving the way for further optimizations in performance. The passively Q-switched laser operation of Dy-doped fluoride fiber is achieved employing a semiconductor saturable absorber mirror for the first time, demonstrating a stable operation with a minimum pulse duration of 580 ns, a highest repetition frequency of 103 kHz and a pulse energy up to 300 nJ

Tunable 30 fs light pulses at 1 W power level from a Yb-pumped optical parametric oscillator

We report on a Yb-pumped optical parametric oscillator (OPO) that delivers 30 fs pulses with spectral coverage from 680 to 910 nm and an average output power of up to 1.1 W. The resulting peak power is â\u88¼0.5 MW, which is, to the best of our knowledge, the highest ever demonstrated in a femtosecond OPO. The intensity noise remains at a level of 0.2% rms, and rapid wavelength tuning is obtained by simply scanning the resonator length. The performances of the OPO are promising for a variety of applications in nonlinear microscopy and ultrafast spectroscopy